Yoko Kanno's work is gold, check out Macross Plus OST entire soundtrack is amazing with Voices being the top song and most iconic.
Alot of electronic symphonic sounds in the stuff composed for the "Virtual Idol" character (in 1995 they were predicting such things as the holographic virtual pop star) and it has some great beats and vocals. Very sort of experimental feeling in over all.
One of the top anime soundtracks of all times, if not a top all time soundtrack.
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