Reload, and I'm not trolling. 2nd would probably be And Justice For All and 3rd would be Garage Inc.
I think Hetfield was in better vocal form on Reload than he ever was before or has been since. I also think the album (mostly) consists of well-written alternative rock tunes with a lot of good guitar work. Fuel and the Memory Remains are completely skippable, but there's so much great stuff late on the album. Fixxxer just may be their best song!
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